Ferroelasticity in palmierite-type (1 - x)Pb3(PO4)2- xPb3(AsO4)2

Link:
Autor/in:
Erscheinungsjahr:
2017
Medientyp:
Text
Schlagworte:
  • ferroelastic
  • twinning
  • domains
  • x-ray diffraction
  • Raman spectroscopy
Beschreibung:
  • Lead phosphate–arsenate Pb3(P1−x As x O4)2 undergoes an improper ferroelastic phase transition from a rhombohedral paraphase $R\bar{3}m$ to a monoclinic ferrophase $C2/c$ leading to distinct twin boundary patterns. On cooling compounds with x larger than 0.8 undergo further transitions to monoclinic low-temperature phases, whereas the composition with x  =  0.8 shows order-parameter coupling phenomena. The transformation $R\bar{3}m$ –$C2/c$ was described on the basis of a three-state Potts model and the existence of precursors of monoclinic clusters in the rhombohedral paraphase. The system is one of the best studied improper ferroelastics. Due to its two-mode phonon behaviour the solid solution exhibits multistep temperature- as well as pressure-driven structural transformations with different length and time scales. Relevant investigations and findings of this palmierite-type material have been made by Prof E K H Salje. Some of the most prominent results from x-ray diffraction, optical microscopy and Raman scattering are reviewed, and the potential implications for domain-wall structures and engineering are discussed.
Lizenz:
  • info:eu-repo/semantics/closedAccess
Quellsystem:
Forschungsinformationssystem der UHH

Interne Metadaten
Quelldatensatz
oai:www.edit.fis.uni-hamburg.de:publications/6d407e97-252f-4e30-bb52-72d095c7dc40