High Resolution Multiphoton Spectroscopy by a Tunable Free-Electron-Laser Light

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Erscheinungsjahr:
2014
Medientyp:
Text
Beschreibung:
  • Seeded free electron lasers theoretically have the intensity, tunability, and resolution required for multiphoton spectroscopy of atomic and molecular species. Using the seeded free electron laser FERMI and a novel detection scheme, we have revealed the two-photon excitation spectra of dipole-forbidden doubly excited states in helium. The spectral profiles of the lowest (−1,0)+1 1Se and (0,1)0 1De resonances display energy shifts in the meV range that depend on the pulse intensity. The results are explained by an effective two-level model based on calculated Rabi frequencies and decay rates.
Lizenz:
  • info:eu-repo/semantics/closedAccess
Quellsystem:
Forschungsinformationssystem der UHH

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oai:www.edit.fis.uni-hamburg.de:publications/81623463-44a4-4c04-9895-df9932c8a09d