Magnetic-order induced spectral-weight redistribution in La0.7⁢(Sr,Ca)0.3⁢MnO3

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Erscheinungsjahr:
2006
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  • We present the optical and magneto-optical characterization of La0.7⁢(Sr,Ca)0.3⁢MnO3 at temperatures 25K⩽⩽470K. The metal-insulator transition is accompanied by a magnetic-order induced spectral-weight redistribution within 0.5–5.5eV. Relating the kinetic energy of superexchange and double-exchange models to the optical spectral weight allows the distinction of Mn intersite from O⁢2⁢→Mn⁢3⁢ charge-transfer excitations. We infer that with decreasing temperature, the lower Hubbard band approaches the in-gap states by a reduction of the Jahn-Teller energy causing the metal-insulator transition. We estimate ⁢≈0.8eV, >0.8eV, >2.9eV, and ⩽2.2eV.
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  • info:eu-repo/semantics/closedAccess
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Forschungsinformationssystem der UHH

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oai:www.edit.fis.uni-hamburg.de:publications/d07a4ee6-141a-4766-a483-a76dde45abef