Spin–orbit effects in atomic high-harmonic generation

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Autor/in:
Erscheinungsjahr:
2014
Medientyp:
Text
Schlagworte:
  • high-harmonic generation
  • multiorbital physics
  • spin-orbit coupling
Beschreibung:
  • Spin-orbit interactions lead to small energy gaps between the outermost p1/2 and p3/2 shells of noble gas atoms. Strong-field pulses tunnel-ionize an electron out of either shell resulting in spin-orbit-driven hole motion. These hole dynamics affect the high-harmonic generation (HHG) yield. However, the spectral shape as well as the angular distribution of the HHG emission is not influenced by spin-orbit coupling. We demonstrate the spin-orbit effect on atomic krypton by solving the multi-electron Schrödinger equation with the time-dependent configuration-interaction singles approach. We also provide pulse parameters where this effect can be identified in experiments through an enhancement in the HHG yield as the wavelength of the strong-field pulse increases. © 2014 IOP Publishing Ltd.
Lizenz:
  • info:eu-repo/semantics/restrictedAccess
Quellsystem:
Forschungsinformationssystem der UHH

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oai:www.edit.fis.uni-hamburg.de:publications/248d60cc-e289-4e6d-adf1-8aa2a571ff12