Building principle of triatomic trilobite Rydberg molecules

Link:
Autor/in:
Erscheinungsjahr:
2019
Medientyp:
Text
Beschreibung:
  • We investigate triatomic molecules that consist of two ground-state atoms and a highly excited Rydberg atom, bound at large internuclear distances of thousands of angstroms. In the molecular state the Rydberg electron is in a superposition of high angular momentum states whose probability densities resemble the form of trilobite fossils. The associated potential-energy landscape has an oscillatory shape and supports a rich variety of stable geometries with different bond angles and bond lengths. Based on an electronic structure investigation we analyze the molecular geometry systematically and develop a simple building principle that predicts the triatomic equilibrium configurations. As a representative example we focus on Rb87 trimers correlated to the n=30 Rydberg state. Using an exact diagonalization scheme we determine and characterize localized vibrational states in these potential minima with energy spacings on the order of 100 MHz×h.
Lizenz:
  • info:eu-repo/semantics/restrictedAccess
Quellsystem:
Forschungsinformationssystem der UHH

Interne Metadaten
Quelldatensatz
oai:www.edit.fis.uni-hamburg.de:publications/4527d946-ef04-42d3-a9bd-bcbaf109836c