Fundamental difference between measured and calculated exciton-phonon coupling in nanostructures

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Erscheinungsjahr:
2019
Medientyp:
Text
Beschreibung:
  • Using ab initio density functional theory applied to semiconductor nanoclusters, we show that optical experiments where absorption is involved probe vibrations that are not necessarily the ones with large exciton-phonon matrix elements. The vibrations involved in these experiments must satisfy more stringent symmetry constraints than given by the selection rules of the exciton-phonon matrix elements. This resolves a long-standing observed discrepancy, while offering a viable theoretical approach to properly account for the experimental situation.
Lizenz:
  • info:eu-repo/semantics/restrictedAccess
Quellsystem:
Forschungsinformationssystem der UHH

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oai:www.edit.fis.uni-hamburg.de:publications/00a441d7-312d-4aa3-b491-082f0b4811d7