Will Ar-37 emissions from light water power reactors become an obstacle to its use for nuclear explosion monitoring?

Link:
Autor/in:
Erscheinungsjahr:
2020
Medientyp:
Text
Schlagworte:
  • Nuclear Test
  • Underground Nuclear Explosions
  • Treaty Organization
  • Radon
  • Radioisotopes
  • Radioactivity
  • 37Ar production routes
  • Treaty verification
  • PWR
  • Anthropogenic background
  • CTBT
  • 37Ar
  • Nuclear Test
  • Underground Nuclear Explosions
  • Treaty Organization
  • Radon
  • Radioisotopes
  • Radioactivity
Beschreibung:
  • 37Ar is a promising candidate for complementing radioxenon isotopes as indicators of underground nuclear explosions. This study evaluates its potential anthropogenic background caused by emissions from commercial pressurized water reactors. Various 37Ar production pathways, which result from activation of 36Ar and of 40Ca, respectively, are identified and their emissions quantified. In-core processes include (1) the restart of operation and degassing of the primary cooling water after maintenance and refueling shutdown, (2) the replacement of primary coolant water for limiting its tritium concentrations, and (3) the leakage of 37Ar produced from calcium impurities in UO2 after fuel rod failures. Activation of air and of calcium in concrete within the biological shield are major out-of-core production pathways. Whereas emissions from in-core processes are transient, a rather constant 37Ar source term results from its out-of-core production. Generic atmospheric dispersion simulations indicate that already at moderate distances from the emitter, concentrations of 37Ar caused by routine reactor operations are far below its cosmogenic background in air. The only exception results from an inadvertent reactor re-start without operation of the primary cooling water degassing system for prolonged time. Such an event also causes high emissions of 41Ar which can be used for discriminating its 37Ar signal from an underground nuclear explosion.
Lizenz:
  • info:eu-repo/semantics/restrictedAccess
Quellsystem:
Forschungsinformationssystem der UHH

Interne Metadaten
Quelldatensatz
oai:www.edit.fis.uni-hamburg.de:publications/7de15396-81ee-496a-a3bc-ae069680127c