Ring–Ring Equilibration in Solid, Even-Numbered Cyclic Poly(l-lactide)s and their Stereocomplexes

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Autor/in:
Erscheinungsjahr:
2020
Medientyp:
Text
Schlagworte:
  • Dilactide
  • 2-Hydroxybutyric Acid
  • Wide-Angle X-Ray Scattering
  • Polypropylenes
  • Lactic Acid
  • Blending
  • Dilactide
  • 2-Hydroxybutyric Acid
  • Wide-Angle X-Ray Scattering
  • Polypropylenes
  • Lactic Acid
  • Blending
Beschreibung:
  • Even-numbered cyclic poly(d-lactide) and poly(l-lactide) are prepared by ring-expansion polymerization. The cyclic pol(l-lactide) is annealed either at 120 or at 160 °C for several days. The progress of transesterification in the solid state is monitored by the formation of odd-numbered cycles via matrix-assisted laser desorption/ionization-time of flight mass spectrometry. The changes of the crystallinity are monitored by differential scanning calorimetry, wide- and small-angle x-ray scattering (WAXS and SAXS) measurements. Despite total even-odd equilibration at 160 °C, the crystallinity of poly(l-lactide) is not reduced. Furthermore, the crystallinity of the stereocomplexes of both cyclic polylactides do not decrease or vanish, as expected, when a blocky or random stereosequence is formed by transesterification. This conclusion is confirmed by 13C NMR spectroscopy. These measurements demonstrate that transesterification is a ring–ring equilibration involving the loops on the surfaces of the lamellar crystallites thereby improving crystallinity and 3D packing of crystallites without significant broadening of the molecular weight distribution.
Lizenz:
  • info:eu-repo/semantics/openAccess
Quellsystem:
Forschungsinformationssystem der UHH

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oai:www.edit.fis.uni-hamburg.de:publications/2e444533-ea02-4852-b22f-022fe518e681