X-ray Raman scattering: a building block for nonlinear spectroscopy

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Autor/in:
Erscheinungsjahr:
2019
Medientyp:
Text
Schlagworte:
  • X-ray free-electron laser
  • nonlinear spectroscopy
  • amplified spontaneous emission
  • resonant inelastic X-ray scattering
  • Raman scattering
Beschreibung:
  • Ultraintense X-ray free-electron laser pulses of attosecond duration can enable new nonlinear X-ray spectroscopic techniques to observe coherent electronic motion. The simplest nonlinear X-ray spectroscopic concept is based on stimulated electronic X-ray Raman scattering. We present a snapshot of recent experimental achievements, paving the way towards the goal of realizing nonlinear X-ray spectroscopy. In particular, we review the first proof-of-principle experiments, demonstrating stimulated X-ray emission and scattering in atomic gases in the soft X-ray regime and first results of stimulated hard X-ray emission spectroscopy on transition metal complexes. We critically asses the challenges that have to be overcome for future successful implementation of nonlinear coherent X-ray Raman spectroscopy.
Lizenz:
  • info:eu-repo/semantics/restrictedAccess
Quellsystem:
Forschungsinformationssystem der UHH

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oai:www.edit.fis.uni-hamburg.de:publications/2b3cbcb5-8f45-44f2-929e-eb261fc1614d