Time-resolved x-ray photoelectron spectroscopy at FLASH

Link:
Autor/in:
Erscheinungsjahr:
2012
Medientyp:
Text
Schlagworte:
  • Charge density waves
  • Charge density
  • Transition metals
  • Superconductors (Materials)
  • Superconducting Materials
  • Superconductivity
  • Charge density waves
  • Charge density
  • Transition metals
  • Superconductors (Materials)
  • Superconducting Materials
  • Superconductivity
Beschreibung:
  • The technique of time-resolved pump-probe x-ray photoelectron spectroscopy using the free-electron laser in Hamburg (FLASH) is described in detail. Particular foci lie on the macrobunch resolving detection scheme, the role of vacuum space-charge effects and the synchronization of pump and probe lasers. In an exemplary case study, the complete Ta 4f core-level dynamics in the layered charge-density-wave (CDW) compound 1T-TaS2 in response to impulsive optical excitation is measured on the sub-picosecond to nanosecond timescale. The observed multi-component dynamics is related to the intrinsic melting and reformation of the CDW as well as to extrinsic pump-laser-induced vacuum space-charge effects.
Lizenz:
  • info:eu-repo/semantics/openAccess
Quellsystem:
Forschungsinformationssystem der UHH

Interne Metadaten
Quelldatensatz
oai:www.edit.fis.uni-hamburg.de:publications/f55ec76e-c830-41a4-910e-5e40ec5fa806