High: Tm poly(L-lactide)s via REP or ROPPOC of L-lactide

Link:
Autor/in:
Erscheinungsjahr:
2020
Medientyp:
Text
Schlagworte:
  • Polystyrene Derivative
  • Polymer Melts
  • Dilactide
  • Block Copolymers
  • Micelles
  • Polymers
  • Polystyrene Derivative
  • Polymer Melts
  • Dilactide
  • Block Copolymers
  • Micelles
  • Polymers
Beschreibung:
  • A new kind of high melting (HTm) pol(l-lactide) was discovered when cyclic poly(l-lactide)s were prepared by ring-expansion polymerization with cyclic tin catalysts at 130-160 °C in bulk. By DSC measurements with 10 K min-1 melting temperatures (Tm) in the range of 190-196 °C were found. The WAXS and SAXS measurements evidenced that not a new crystal lattice but a well-ordered morphology and a higher perfection of the crystallites are responsible for the high Tm values and high crystallinities. Under identical reaction conditions SnOct2-catalyzed and alcohol-initiated ROPs do not yield these crystallites. Furthermore, it was found that the standard crystallites are kinetically favored upon rapid crystallization, whereas the high melting form of poly(l-lactide) is thermodynamically more stable.
Lizenz:
  • info:eu-repo/semantics/openAccess
Quellsystem:
Forschungsinformationssystem der UHH

Interne Metadaten
Quelldatensatz
oai:www.edit.fis.uni-hamburg.de:publications/3c37908b-f4a3-4718-9c32-6b1ab7f8c32d